I'll have to admit also, while a 75 is a great sized tank, I feel that its too small to house a group of pygo's for the long run.
Alot of people have tried Nattereri (usually in groups of 3 or 4). Some have had success, and some not.
Natts are the only one I would do this with. Caribe just grow too large. Its not unusual for juvenile Caribe's to make it to 12" + having been properly cared for. Three caribe at even 9" or 10" would scare me in a 75 gallon, of course this would take a little time, but nowhere near a serra's growth speed.
And I know you love that driftwood, I would too, but it would have to go to make room for swimming. Or at leat cut down.
If your looking to keep a piranha in this tank for the long run, I'd reccomend going with a solitary species, pygo or serra. With the right fish, it would never be sitting still. Constantly patroling his tank.
I'm now trying to decide what I'm going to get next. I'm back and forth about it. A month ago it was a Manny. Now I'm dead set on a solitary Piraya with high redish-orange flames.